将CO2大规模转化为甲醇在可持续经济中具有重要意义。ZrO2因其在CO2吸附和活化方面的出色性能而被认为是Cu基催化剂中的重要载体。然而，在反应过程中Zr物种的演变以及它们的结构对反应途径的影响仍然不清楚。

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